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101.
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David T. Johnston James Farquhar Yanan Shen Andrew L. Masterson 《Geochimica et cosmochimica acta》2008,72(17):4278-4290
Previous geochemical and biomarker studies of the late Paleo-Mesoproterozoic propose a stratified world, with strongly reducing (possibly sulfidic) deep-ocean conditions overlain by an oxygenated surface-ocean and atmosphere. To investigate such a scenario, we look to the structure of the biogeochemical sulfur cycle. We present sulfur (32S, 33S, 34S, and 36S in sulfides) isotope data from the McArthur Basin (Barney Creek, Reward, Velkerri, and McMinn formations) that allows for a direct evaluation of the surface biosphere. We are interested in investigating the types of information that can be gained by including 33S and 36S. When the 34S/32S fractionations are small, the inclusion of 33S and 36S provides little additional information, but does provide ancillary evidence for relative isotopic homogeneity (with the internal consistency of 33S/32S and 36S/32S). When the 34S/32S fractionations are large, direct information about the fractionation mechanisms can be obtained, with the potential to distinguish the biological from abiological processes. For example, the reconstruction of the Roper Group suggests that seawater sulfate concentrations were high enough to buffer against spatial heterogeneities. Overall, our findings agree with previously proposed redox structure of the Proterozoic ocean, highlight contributions from the oxidative sulfur cycle, and outline a new tool for interpreting the state of the surface sulfur cycle. 相似文献
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Stela Cuna Elise Pendall John B. Miller Pieter P. Tans Ed Dlugokencky James W.C. White 《Applied Geochemistry》2008
The Danube Delta-Black Sea region of Romania is an important wetland, and this preliminary study evaluates the significance of this region as a source of atmospheric CH4. Measurements of the mixing ratio and δ13C in CH4 are reported from air and water samples collected at eight sites in the Danube Delta. High mixing ratios of CH4 were found in air (2500–14,000 ppb) and dissolved in water samples (∼1–10 μmol L−1), demonstrating that the Danube Delta is an important natural source of CH4. The intercepts on Keeling plots of about −62‰ show that the main source of CH4 in this region is microbial, probably resulting primarily from acetate fermentation. Atmospheric CH4 and CO data from the NOAA/ESRL (National Oceanic and Atmospheric Administration/Earth System Research Laboratory) were used to make a preliminary estimate of biogenic CH4 at the Black Sea sampling site at Constanta (BSC). These data were used to calculate ratios of CH4/CO in air samples, and using an assumed CH4/CO anthropogenic emissions ratio of 0.6, fossil fuel emissions at BSC were estimated. Biogenic CH4 emissions were then estimated by a simple mass balance approach. Keeling plots of well-mixed air from the BSC site suggested a stronger wetland source in summer and a stronger fossil fuel source in winter. 相似文献
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Ron Johnston Derek Gregory Geraldine Pratt Michael Watts Sarah Whatmore 《Geoforum》2008,39(3):1105-1107
A reply to a recent paper by Setten. 相似文献
108.
W. E. Featherstone J. F. Kirby A. H. W. Kearsley J. R. Gilliland G. M. Johnston J. Steed R. Forsberg M. G. Sideris 《Journal of Geodesy》2001,75(5-6):313-330
The AUSGeoid98 gravimetric geoid model of Australia has been computed using data from the EGM96 global geopotential model,
the 1996 release of the Australian gravity database, a nationwide digital elevation model, and satellite altimeter-derived
marine gravity anomalies. The geoid heights are on a 2 by 2 arc-minute grid with respect to the GRS80 ellipsoid, and residual
geoid heights were computed using the 1-D fast Fourier transform technique. This has been adapted to include a deterministically
modified kernel over a spherical cap of limited spatial extent in the generalised Stokes scheme. Comparisons of AUSGeoid98
with GPS and Australian Height Datum (AHD) heights across the continent give an RMS agreement of ±0.364 m, although this apparently
large value is attributed partly to distortions in the AHD.
Received: 10 March 2000 / Accepted: 21 February 2001 相似文献
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Global warming due to increased concentrations of atmospheric CO2 is expected to be amplified in middle and higher latitudes. Consequently, ecosystems in these latitudes will experience more pronounced climatic variations. This investigation attempts to assess the sensitivity of Canada's ecosystems to climatic change. Potential ecological impacts resulting from global warming are outlined. With this background, the effects of a doubled CO2 climate are applied to a classification model derived from the current ecological setting. Results reveal not only major shifts in ecological boundaries but also changes in the character of these broadly distributed ecosystems. 相似文献